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This is the peer reviewed version of the following article: Shi, W., Liu, X., Deng, T., Huang, S., Ding, M., Miao, X., Zhu, C., Zhu, Y., Liu, W., Wu, F., Gao, C., Yang, S.‐W., Yang, H. Y., Shen, J., Cao, X., Enabling Superior Sodium Capture for Efficient Water Desalination by a Tubular Polyaniline Decorated with Prussian Blue Nanocrystals. Adv. Mater. 2020, 32, 1907404. https://doi.org/10.1002/adma.201907404, which has been published in final form at 10.1002/adma.201907404. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Use of Self-Archived Versions